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Diffusion-enhanced exciton dissociation in single-material organic solar cells

Tijdschriftbijdrage - Tijdschriftartikel

Single-material organic solar cells have recently attracted research attention due to their simplicity, morphological robustness and high yield of exciton dissociation. Using alpha-sexithiophene as a model system, we show that the single-event probability of the exciton dissociation at the boundaries of polycrystalline domains with different molecular orientation is extremely low (similar to 0.5%), while a high efficiency of charge generation is gained via hundred-fold crossings of the domain boundaries due to the long exciton diffusion length (similar to 45 nm).
Tijdschrift: PCCP. Physical chemistry chemical physics (Print)
ISSN: 1463-9076
Issue: 37
Volume: 23
Pagina's: 20848 - 20853
Jaar van publicatie:2021
BOF-keylabel:ja
IOF-keylabel:ja
BOF-publication weight:2
Auteurs:International
Authors from:Higher Education
Toegankelijkheid:Open